If your project is going to be in c++ , go for qt though Gtk also has bindings for C++ (Gtkmm). Qt has good cross platform support and will serve your purpose . You can use qt-designer coupled with Kdevelop for a complete IDE. for gtk Glade and anjuta will be the combo. Maybe u can try some simple apps in both and check for yourself which one you like more or suits you. There is good documentation with qt and even fro gtk there are good startup tutorials on gtk.org.
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